Abstract

Coal-fired power plants cause serious environmental impacts associated with air pollution, particulate matter, and heavy metals (HMs), among others. In this work, the spatial, temporal, and vertical concentration variations, pollution indices, and sources of As, Cr, Cd, Pb, Hg, Fe, Mn, Cu, Zn, and Ni heavy metals were studied in the surface soil of the largest coal-burning area in India (Korba Basin) from 2011 to 2015. Heavy metal concentrations were in the following ranges: 49164  mgkg1 (As and Cr), 0.110.56  mgkg1 (Cd), 72194  mgkg1 (Pb), and 0.110.39  mgkg1 (Hg). Pollution indices showed a very severe contamination, especially for As, Ni, and Pb. In particular, the detected As content in the soil in both arsenite and arsenate forms was several times higher than the permissible limit. Urgent measures are needed to minimize the rate of contamination and remediate the extraordinarily serious heavy metals pollution problem in this area.

Get full access to this article

View all available purchase options and get full access to this article.

Acknowledgments

The University Grant Commission, New Delhi, is greatly acknowledged for awarding the BSR fellowship to the fourth author through Grant No. F.18-1/2011(BSR)2016.

References

Agarwal, T. 2009. “Concentration level, pattern and toxic potential of PAHs in traffic soil of Delhi, India.” J. Hazard. Mater. 171 (1–3): 894–900. https://doi.org/10.1016/j.jhazmat.2009.06.081.
Agrawal, P., A. Mittal, R. Prakash, M. Kumar, T. B. Singh, and S. K. Tripathi. 2010. “Assessment of contamination of soil due to heavy metals around coal fired thermal power plants at Singrauli region of India.” Bull. Environ. Contam. Toxicol. 85 (2): 219–223. https://doi.org/10.1007/s00128-010-0043-8.
ATSDR (Agency for Toxic Substances and Disease Registry). 2000. Toxicological profile for chromium. Atlanta: Health Administration Press.
Bahloul, M., H. Baati, R. Amdouni, and C. Azri. 2018. “Assessment of heavy metals contamination and their potential toxicity in the surface sediments of Sfax Solar Saltern, Tunisia.” Environ. Earth Sci. 77 (1): 27. https://doi.org/10.1007/s12665-018-7227-7.
Bhuiyan, M. A., L. Parvez, M. A. Islam, S. B. Dampare, and S. Suzuki. 2010. “Heavy metal pollution of coal mine-affected agricultural soils in the northern part of Bangladesh.” J. Hazard. Mater. 173 (1–3): 384–392. https://doi.org/10.1016/j.jhazmat.2009.08.085.
Cheng, C.-H., J. Lehmann, J. Kinyangi, D. Solomon, and T.-L. Wu. 2010. “Long-term effects of black carbon on soil properties.” In Proc., 19th World Congress of Soil Science, Soil Solutions for a Changing World. Brisbane, Australia: International Union of Soil Sciences.
Chrysikou, L., P. Gemenetzis, A. Kouras, E. Manoli, E. Terzi, and C. Samara. 2008. “Distribution of persistent organic pollutants, polycyclic aromatic hydrocarbons and trace elements in soil and vegetation following a large scale landfill fire in northern Greece.” Environ. Int. 34 (2): 210–225. https://doi.org/10.1016/j.envint.2007.08.007.
Crommentuijn, T., M. D. Polder, and E. J. Van de Plassche. 1997. Maximum permissible concentrations and negligible concentrations for metals, Taking background concentrations into account. Bilthoven, Netherlands: Rijksinstituut voor Volksgezondheid en Milieu.
Dragović, S., M. Ćujić, L. Slavković-Beškoski, B. Gajić, B. Bajat, M. Kilibarda, and A. Onjia. 2013. “Trace element distribution in surface soils from a coal burning power production area: A case study from the largest power plant site in Serbia.” Catena 104: 288–296. https://doi.org/10.1016/j.catena.2012.12.004.
EPA. 2007. Human and ecological risk assessment of coal combustion wastes. Washington, DC: Office of Solid Waste.
Hamilton, G. A., and H. E. Hartnett. 2013. “Soot black carbon concentration and isotopic composition in soils from an arid urban ecosystem.” Org. Geochem. 59: 87–94. https://doi.org/10.1016/j.orggeochem.2013.04.003.
Han, Y. M., B. A. M. Bandowe, C. Wei, J. J. Cao, W. Wilcke, G. H. Wang, H. Y. Ni, Z. D. Jin, Z. S. An, and B. Z. Yan. 2015. “Stronger association of polycyclic aromatic hydrocarbons with soot than with char in soils and sediments.” Chemosphere 119: 1335–1345. https://doi.org/10.1016/j.chemosphere.2014.02.021.
Han, Y. M., J. J. Cao, J. C. Chow, J. G. Watson, Z. S. An, and S. X. Liu. 2009. “Elemental carbon in urban soils and road dusts in Xi’an, China and its implication for air pollution.” Atmos. Environ. 43 (15): 2464–2470. https://doi.org/10.1016/j.atmosenv.2009.01.040.
He, Y., and G. L. Zhang. 2009. “Historical record of black carbon in urban soils and its environmental implications.” Environ. Pollut. 157 (10): 2684–2688. https://doi.org/10.1016/j.envpol.2009.05.019.
Huang, X., J. Hu, F. Qin, W. Quan, R. Cao, M. Fan, and X. Wu. 2017. “Heavy metal pollution and ecological assessment around the Jinsha coal-fired power plant (China).” Int. J. Environ. Res. Public Health 14 (12): 1589. https://doi.org/10.3390/ijerph14121589.
Khan, M. H. R., A. Ashraf, A. A. Seddique, A. Rahman, and Y. Shimizu. 2017. “Heavy metals contamination assessment of water and soils in and around Barapukuria coal mine area, Bangladesh.” Am. J. Environ. Prot. 6 (4): 80–86. https://doi.org/10.11648/j.ajep.20170604.11.
Kwon, J. C., Z. D. Nejad, and M. C. Jung. 2017. “Arsenic and heavy metals in paddy soil and polished rice contaminated by mining activities in Korea.” Catena 148: 92–100. https://doi.org/10.1016/j.catena.2016.01.005.
Li, R., J. Ding, W. Fu, L. Gan, and Y. Li. 2017. “Mercury pollutions in vegetables, grains and soils from areas surrounding coal-fired power plants.” Sci. Rep. 7: 46545. https://doi.org/10.1038/srep46545.
Liang, B., et al. 2006. “Black carbon increases cation exchange capacity in soils.” Soil Sci. Soc. Am. J. 70 (5): 1719–1730. https://doi.org/10.2136/sssaj2005.0383.
Liu, S., X. Xia, Y. Zhai, R. Wang, T. Liu, and S. Zhang. 2011. “Black carbon (BC) in urban and surrounding rural soils of Beijing, China: Spatial distribution and relationship with polycyclic aromatic hydrocarbons (PAHs).” Chemosphere 82 (2): 223–228. https://doi.org/10.1016/j.chemosphere.2010.10.017.
Muller, G. 1969. “Index of geo-accumulation in sediments of the Rhine River.” J. Geol. 2 (3): 108–118.
Munawer, M. E. 2018. “Human health and environmental impacts of coal combustion and post-combustion wastes.” J. Sustainable Min. 17 (2): 87–96. https://doi.org/10.1016/j.jsm.2017.12.007.
Nagajyoti, P. C., K. D. Lee, and T. V. M. Sreekanth. 2010. “Heavy metals, occurrence and toxicity for plants: A review.” Environ. Chem. Lett. 8 (3): 199. https://doi.org/10.1007/s10311-010-0297-8.
Nam, J. J., O. Gustafsson, P. K. Karakus, K. Breivik, E. Steinnes, and K. C. Jones. 2008. “Relationships between organic matter, black carbon and persistent organic pollutants in European background soils: Implications for sources and environmental fate.” Environ. Pollut. 156 (3): 809–817. https://doi.org/10.1016/j.envpol.2008.05.027.
Özkul, C. 2016. “Heavy metal contamination in soils around the Tunçbilek Thermal power plant (Kütahya, Turkey).” Environ. Monit. Assess. 188 (5): 284. https://doi.org/10.1007/s10661-016-5295-2.
Pandey, B., M. Agrawal, and S. Singh. 2016. “Ecological risk assessment of soil contamination by trace elements around coal mining area.” J. Soils Sediments 16 (1): 159–168. https://doi.org/10.1007/s11368-015-1173-8.
Patel, K. S., R. Sharma, N. S. Dahariya, R. K. Patel, B. Blazhev, and L. Matini. 2016. “Black carbon and heavy metal contamination of soil.” Pol. J. Environ. Stud. 25 (2): 717–724. https://doi.org/10.15244/pjoes/61062.
Rudnick, R. L., and S. Gao. 2003. “The composition of the continental crust.” Chap. 3.01 in Vol. 3 of Treatise on geochemistry, edited by H. D. Holland and K. K. Turekian, 1–64. Oxford, UK: Elsevier.
Sengupta, S., T. Chatterjee, P. B. Ghosh, and T. Saha. 2010. “Heavy metal accumulation in agricultural soils around a coal fired thermal power plant (Farakka) in India.” J. Environ. Sci. Eng. 52 (4): 299–306.
Sharma, R., K. S. Patel, L. Lata, and H. Milosh. 2017. “Contamination of pond water and sediment in coal burning area.” J. Environ. Prot. 8 (3): 358–379. https://doi.org/10.4236/jep.2017.83027.
Sinex, S. A., and G. R. Helz. 1981. “Regional geochemistry of trace elements in Chesapeake Bay sediments.” Environ. Geol. 3 (6): 315–323. https://doi.org/10.1007/BF02473521.
Singh, R., D. P. Singh, N. Kumar, S. K. Bhargava, and S. C. Barman. 2010. “Accumulation and translocation of heavy metals in soil and plants from fly ash contaminated area.” J. Environ. Biol. 31 (4): 421–430.
Stafilova, T., R. Sajnb, M. Arapceskac, I. Kungulovskid, and J. Alijagi. 2018. “Geochemical properties of topsoil around the coal mine and thermoelectric power plant.” J. Environ. Sci. Health: Part A 53 (9): 1–16. https://doi.org/10.1080/10934529.2018.1445076.
Su, C., L. Q. Jiang, and W. J. Zhang. 2014. “A review on heavy metal contamination in the soil worldwide: Situation, impact and remediation techniques.” Environ. Skeptics Critics 3 (2): 24–38.
Suna, L., D. Guoa, K. Liua, H. Menga, Y. Zhenga, F. Yuana, and G. Zhub. 2019. “Levels, sources, and spatial distribution of heavy metals in soils from a typical coal industrial city of Tangshan, China.” Catena 175: 101–109. https://doi.org/10.1016/j.catena.2018.12.014.
Tan, K. H. 2005. Soil sampling, preparation and analysis. 2nd ed. Boca Raton, FL: CRC Press.
Tanić, M. N., M. R. Ćujić, B. A. Gajić, M. Z. Daković, and S. D. Dragović. 2018. “Content of the potentially harmful elements in soil around the major coal-fired power plant in Serbia: Relation to soil characteristics, evaluation of spatial distribution and source apportionment.” Environ. Earth Sci. 77 (1): 28. https://doi.org/10.1007/s12665-017-7214-4.
Tchounwou, P. B., C. G. Yedjou, A. K. Patlolla, and D. J. Sutton. 2012. “Heavy metal toxicity and the environment.” In Vol. 101 of Molecular, clinical and environmental toxicology, experientia supplementum, edited by A. Luch. Basel, Switzerland: Springer.
Tomlinson, D. L., J. G. Wilson, C. R. Harris, and D. W. Jeffrey. 1980. “Problem in assessment of heavy-metal levels in estuaries and the formation of a pollution index.” Helgoländer Meeres 33 (1–4): 566–575. https://doi.org/10.1007/BF02414780.
VDI German. 1997. Measurement of soot (emission) thermographic analysis of elemental carbon by thermal desorption of organic carbon. Düsseldorf, Germany: VDI German.
Wang, X. S. 2010. “Black carbon in urban top soils of Xuzhou (China): Environmental implication and magnetic proxy.” Environ. Monit. Assess. 163 (1–4): 41–47. https://doi.org/10.1007/s10661-009-0814-z.
Wang, X. S., P. Zhang, H. Y. Zhou, and J. Fu. 2012. “Association of black carbon with polycyclic aromatic hydrocarbons and heavy metals in urban top soils and environmental implications.” Int. J. Environ. Stud. 69 (5): 705–713. https://doi.org/10.1080/00207233.2012.702414.
Wang, X.-S., and Y. Qin. 2007. “Some characteristics of the distribution of heavy metals in urban topsoil of Xuzhou, China.” Environ. Geochem. Health 29 (1): 11–19. https://doi.org/10.1007/s10653-006-9052-2.
Zhang, K., C. Qiang, and J. Liu. 2018. “Spatial distribution characteristics of heavy metals in the soil of coal chemical industrial areas.” J. Soils Sediments 18 (5): 2044–2052. https://doi.org/10.1007/s11368-018-1972-9.
Zhao, J., X. Shi, V. Castranova, and M. Ding. 2009. “Occupational toxicology of nickel and nickel compounds.” J. Environ. Pathol. Toxicol. Oncol. 28 (3): 177–208. https://doi.org/10.1615/JEnvironPatholToxicolOncol.v28.i3.10.
Zong, Y., Q. Xiao, and S. Lu. 2016. “Black carbon (BC) of urban topsoil of steel industrial city (Anshan), northeastern China: Concentration, source identification and environmental implication.” Sci. Total Environ. 569–570: 990–996. https://doi.org/10.1016/j.scitotenv.2016.06.097.

Information & Authors

Information

Published In

Go to Journal of Hazardous, Toxic, and Radioactive Waste
Journal of Hazardous, Toxic, and Radioactive Waste
Volume 23Issue 4October 2019

History

Received: Mar 15, 2019
Accepted: May 8, 2019
Published online: Aug 9, 2019
Published in print: Oct 1, 2019
Discussion open until: Jan 9, 2020

Permissions

Request permissions for this article.

Authors

Affiliations

Reetu Sharma, Ph.D. [email protected]
School of Studies in Chemistry, Pt. Ravishankar Shukla Univ., Raipur 492010, India. Email: [email protected]
Ankit Yadav [email protected]
School of Studies in Environmental Science, Pt. Ravishankar Shukla Univ., Raipur 492010, India. Email: [email protected]
Shobhana Ramteke [email protected]
Ph.D. Student, School of Studies in Environmental Science, Pt. Ravishankar Shukla Univ., Raipur 492010, India. Email: [email protected]
Khageshwar Singh Patel [email protected]
Professor Emeritus, School of Studies in Chemistry, Pt. Ravishankar Shukla Univ., Raipur 492010, India (corresponding author). Email: [email protected]
Lesia Lata, Ph.D. [email protected]
Dept. of Soil Science, Maria Curie-Skłodowska Univ., Kraśnicka av, 20-718 Lublin, Poland. Email: [email protected]
Huber Milosh [email protected]
Professor, Dept. of Geology, Maria Curie-Skłodowska Univ., Kraśnicka av, 20-718 Lublin, Poland. Email: [email protected]
Warren T. Corns, Ph.D. [email protected]
PS Analytical Ltd., Arthur House, Unit 11 Cray Fields Industrial Estate, Orpington, Kent BR5 3HP, UK. Email: [email protected]
Pablo Martín-Ramos [email protected]
Professor, Dept. of Agricultural and Environmental Sciences, Instituto de Investigación en Ciencias Ambientales de Aragón, Univ. of Zaragoza, Carretera de Cuarte, s/n, 22071 Huesca, Spain. Email: [email protected]

Metrics & Citations

Metrics

Citations

Download citation

If you have the appropriate software installed, you can download article citation data to the citation manager of your choice. Simply select your manager software from the list below and click Download.

Cited by

View Options

Get Access

Access content

Please select your options to get access

Log in/Register Log in via your institution (Shibboleth)
ASCE Members: Please log in to see member pricing

Purchase

Save for later Information on ASCE Library Cards
ASCE Library Cards let you download journal articles, proceedings papers, and available book chapters across the entire ASCE Library platform. ASCE Library Cards remain active for 24 months or until all downloads are used. Note: This content will be debited as one download at time of checkout.

Terms of Use: ASCE Library Cards are for individual, personal use only. Reselling, republishing, or forwarding the materials to libraries or reading rooms is prohibited.
ASCE Library Card (5 downloads)
$105.00
Add to cart
ASCE Library Card (20 downloads)
$280.00
Add to cart
Buy Single Article
$35.00
Add to cart

Get Access

Access content

Please select your options to get access

Log in/Register Log in via your institution (Shibboleth)
ASCE Members: Please log in to see member pricing

Purchase

Save for later Information on ASCE Library Cards
ASCE Library Cards let you download journal articles, proceedings papers, and available book chapters across the entire ASCE Library platform. ASCE Library Cards remain active for 24 months or until all downloads are used. Note: This content will be debited as one download at time of checkout.

Terms of Use: ASCE Library Cards are for individual, personal use only. Reselling, republishing, or forwarding the materials to libraries or reading rooms is prohibited.
ASCE Library Card (5 downloads)
$105.00
Add to cart
ASCE Library Card (20 downloads)
$280.00
Add to cart
Buy Single Article
$35.00
Add to cart

Media

Figures

Other

Tables

Share

Share

Copy the content Link

Share with email

Email a colleague

Share