Technical Papers
Dec 1, 2022

Influence of Soil Heterogeneity on Water Flow and Solute Transport Characterized by Dye Tracer Experiments

Publication: Journal of Hydrologic Engineering
Volume 28, Issue 2

Abstract

Soil heterogeneity is a key factor affecting horizontal water flow and solute transport in unsaturated soil, in which particle distribution, pore structure, and pore connectivity in the soil all present fractal characteristics. The initial water content of soil has significant influence in the resulting heterogeneity of the soil structure, which can affect the water flow and solute transport. In this study, through a series of horizontal transport laboratory simulation experiments in soil columns, the initial water content dependency of transport was elucidated using the fractal Richards’ equation (FRE) model. We first observed that water flows faster in soil columns with higher initial water content, but the law is opposite in the initial process of water flow. By analyzing the variation of parameter values in the FRE model, we speculated that the abnormal phenomenon of early diffusion is caused by the heterogeneity of the soil structure. To elucidate the mechanisms of the water content’s dependency of the solute transport process and to identify the circumstance of altering of flow regime, a series of dye tracer experiments were conducted. Results show that in soil columns with low water content, the inflow of external fluid leads to the agglomeration of soil particles. Combined with matric suction, the heterogeneity of the soil structure is enhanced, which affects the formation of water flow and solute transport paths. It even leads to preferential flow in unsaturated soil columns with low water content.

Get full access to this article

View all available purchase options and get full access to this article.

Data Availability Statement

All data included in this study are available upon request by contact with the corresponding author.

Acknowledgments

Our research has been supported by the National Natural Science Foundation of China (Grant No. 11572112) and the Fundamental Research Funds for the Central Universities (No. 2016B44914). The support of the Experiment Center of Mechanics and Materials in Hohai University is also appreciated.

References

Abd, E. G. E., and J. J. Milczarek. 2004. “Neutron radiography study of water absorption in porous building materials: Anomalous diffusion analysis.” J. Phys. D Appl. Phys. 37 (16): 2305. https://doi.org/10.1088/0022-3727/37/16/013.
Alaoui, A., and B. Goetz. 2008. “Dye tracer and infiltration experiments to investigate macropore flow.” Geoderma 144 (1–2): 279–286. https://doi.org/10.1016/j.geoderma.2007.11.020.
Bartoli, F., R. Philippy, M. Doirisse, S. Niquet, and M. Dubuit. 1991. “Structure and self-similarity in silty and sandy soils: The fractal approach.” Eur. J. Soil Sci. 42 (2): 167–185. https://doi.org/10.1111/j.1365-2389.1991.tb00399.x.
Blumenröder, J., P. Sechet, J. E. Kakkonen, and M. G. J. Hartl. 2017. “Microplastic contamination of intertidal sediments of Scapa Flow, Orkney: A first assessment.” Mar. Pollut. Bull. 124: 112–120. https://doi.org/10.1016/j.marpolbul.2017.07.009.
Bogner, W., and S. Huwe. 2008. “Analysing flow patterns from dye tracer experiments in a forest soil using extreme value statistics.” Eur. J. Soil Sci. 59: 103–113.
Bouma, J., and L. W. Dekker. 1978. “A case study on infiltration into dry clay soil I. Morphological observations.” Geoderma 20 (1): 27–40. https://doi.org/10.1016/0016-7061(78)90047-2.
Bruce, R. R., and A. Klute. 1956. “The measurement of soil moisture diffusivity1.” Soil Sci. Soc. Am. J. 20 (4): 8446–8455. https://doi.org/10.2136/sssaj1956.03615995002000040004x.
Cao, C., D. Yin, G. Xiang, H. Guo, and Y. Chen. 2021. “Study on horizontal diffusion of agent solutions in underground unsaturated soil: Experiments and model simulations.” Environ. Eng. Res. 3 (26): 200119. https://doi.org/10.2136/sssaj1956.03615995002000040004x.
Chen, B., X. Liang, W. Xu, X. Huang, and X. Li. 2012. “The changes in trace metal contamination over the last decade in surface sediments of the Pearl River Estuary, South China.” Sci. Total Environ. 439 (439C): 141–149. https://doi.org/10.1016/j.scitotenv.2012.09.025.
Chen, W. 2006. “Time–space fabric underlying anomalous diffusion.” Chaos Solitons Fractals 28 (4): 923–929. https://doi.org/10.1016/j.chaos.2005.08.199.
Chen, W., L. Yingjie, and Y. Xu. 2018. “Soil infiltration rates and hydrology model Classificatios based on the Hausdorff fractal derivative Richards equation.” Appl. Math. Mech. 39 (1): 77–82. https://doi.org/10.1016/J.CHAOS.2005.08.199.
Coats, K. H., and B. D. Smith. 1964. “Dead-end pore volume and dispersion in porous media.” Soc. Petrol. Eng. J. 4 (1): 73–84. https://doi.org/10.2118/647-PA.
Cushman, J. H., D. O. Malley, and M. Park. 2009. “Anomalous diffusion as modeled by a nonstationary extension of Brownian motion.” Phys. Rev. E: Stat. Nonlinear Soft Matter Phys. 79 (3): 032101. https://doi.org/10.1103/PhysRevE.79.032101.
Droogers, P., A. Stein, J. Bouma, and G. D. Boer. 1998. “Parameters for describing soil macroporosity derived from staining patterns.” Geoderma 83 (3–4): 293–308. https://doi.org/10.1016/S0016-7061(98)00005-6.
Durner, W., and L. Kai. 2006. “Determining soil hydraulic properties.” In Encyclopedia of hydrological sciences. New York: John Wiley & Sons. https://doi.org/10.1002/0470848944.hsa077b.
Elrick, D. E., and L. K. French. 1966. “Miscible displacement patterns on disturbed and undisturbed soil cores.” Soil Sci. Soc. Am. J. 30 (2): 153–156. https://doi.org/10.2136/sssaj1966.03615995003000020007x.
Enell, A., F. Reichenberg, P. Warfvinge, and G. Ewald. 2004. “A column method for determination of leaching of polycyclic aromatic hydrocarbons from aged contaminated soil.” Chemosphere 54 (6): 707–715. https://doi.org/10.1016/j.chemosphere.2003.08.026.
Fan, X., G. Guo, H. Sun, and X. Hao. 2019. “Experimental verification and analysis of fractal Richards’ equation model in describing horizontal water transport in unsaturated soil.” Chin. J. Environ. Eng. 37 (12): 212–217.
Gerolymatou, E., I. Vardoulakis, and R. Hilfer. 2006. “Modelling infiltration by means of a nonlinear fractional diffusion model.” J. Phys. D Appl. Phys. Europhys. J. 39 (18): 1–22. https://doi.org/10.1088/0022-3727/39/18/022.
Guerrini, I. A., and D. Swartzendruber. 1992. “Soil water diffusivity as explicitly dependent on both time and water content.” Soil Sci. Soc. Am. J. 56 (2): 335–340. https://doi.org/10.2136/sssaj1992.03615995005600020001x.
Hamlen, C. J., and R. G. Kachanoski. 2004. “Influence of initial and boundary conditions on solute transport through undisturbed soil columns.” Soil Sci. Soc. Am. J. 68 (2): 404. https://doi.org/10.2136/sssaj2004.4040.
Hangen, E., H. H. Gerke, W. Schaaf, and R. F. Hüttl. 2004. “Flow path visualization in a lignitic mine soil using iodine–starch staining.” Geoderma 120 (1–2): 121–135. https://doi.org/10.1016/j.geoderma.2003.08.011.
Hu, S., H. Zhu, and Y. Chen. 2017. “One-dimensional horizontal infiltration experiment for determining permeability coefficient of loamy sand.” J. Arid Land 9: 27–37. https://doi.org/10.1007/s40333-016-0062-3.
Jalali, M., and D. L. Rowell. 2008. “Prediction leaching of potassium using the convective–dispersive and the convective log-normal transfer function models.” Environ. Geol. 55 (4): 863–874. https://doi.org/10.1007/s00254-007-1038-6.
Jarvis, N. J. 2010. “A review of non-equilibrium water flow and solute transport in soil macropores: Principles, controlling factors and consequences for water quality.” Eur. J. Soil Sci. 58 (3): 523–546. https://doi.org/10.1111/j.1365-2389.2007.00915.x.
Kanchanasut, P., D. Scotter, and R. Tillman. 1978. “Preferential solute movement through larger soil voids. II. Experiments with saturated soil.” Aust. J. Soil Res. 16 (3): 269–276. https://doi.org/10.1071/SR9780269.
Kang, J. B., and C. D. Shackelford. 2011. “Consolidation enhanced membrane behavior of a geosynthetic clay liner.” Geotextiles Geomembr. 29 (6): 544–556. https://doi.org/10.1016/j.geotexmem.2011.07.002.
Kodeová, R., K. Němeek, V. Kode, and A. Igová. 2012. “Using dye tracer for visualization of preferential flow at macro- and microscales.” Vadose Zone J. 11 (1): 1–12. https://doi.org/10.2136/vzj2011.0088.
Küntz, M., and P. Lavallée. 2001. “Experimental evidence and theoretical analysis of anomalous diffusion during water infiltration in porous building materials.” J. Phys. D Appl. Phys. 34 (16): 2547. https://doi.org/10.1088/0022-3727/34/16/322.
Lambe, T. W. 1958. The structure of compacted clay. Reston, VA: ASCE.
Liu, P. W. G., L. M. Whang, M. C. Yang, and S. S. Cheng. 2008. “Biodegradation of diesel-contaminated soil: A soil column study.” J. Chin. Inst. Chem. Eng. 39 (5): 419–428. https://doi.org/10.1016/j.jcice.2008.03.006.
Ma, D. H., M. A. Shao, J. B. Zhang, and Q. J. Wang. 2010. “Validation of an analytical method for determining soil hydraulic properties of stony soils using experimental data.” Geoderma 159 (3–4): 262–269. https://doi.org/10.1016/j.geoderma.2010.08.001.
Markus, W., and N. Felix. 2003. “An experimental tracer study of the role of macropores in infiltration in grassland soils.” Hydrol. Processes 17 (2): 477–493. https://doi.org/10.1002/hyp.1136.
Miao, C. Y. 2007. “Fractal characteristics of soil particles in surface layer of black soil.” Chin. J. Appl. Ecol. 18 (9): 1987–1993.
Öhrström, P., Y. Hamed, M. Persson, and R. Berndtsson. 2004. “Characterizing unsaturated solute transport by simultaneous use of dye and bromide.” J. Hydrol. 289 (1–4): 23–35. https://doi.org/10.1016/j.jhydrol.2003.10.014.
Pachepsky, Y., D. Timlinb, and W. Rawlsc. 2003. “Generalized Richards’ equation to simulate water transport in unsaturated soils.” J. Hydrol. 272 (1–4): 3–13. https://doi.org/10.1016/S0022-1694(02)00251-2.
Padilla, I. Y., T. Yeh, and M. H. Conklin. 1999. “The effect of water content on solute transport in unsaturated porous media.” Water Resour. Res. 35 (11): 3303–3313. https://doi.org/10.1029/1999WR900171.
Parlange, M. B., S. N. Prasad, J. Y. Parlange, and R. Mkens. 1992. “Extension of the Heaslet-Alksne Technique to arbitrary soil water diffusivities.” Water Resour. Res. 28 (10): 2793–2797. https://doi.org/10.1029/92WR01683.
Peyton, R. L., C. J. Gantzer, S. H. Anderson, B. A. Haeffner, and P. Pfeifer. 1994. “Fractal dimension to describe soil macropore structure using X ray computed tomography.” Water Resour. Res. 30 (3): 691–700. https://doi.org/10.1029/93WR02343.
Richards, A. L. 1931. “Capillary conduction of liquids through porous mediums.” J. Appl. Phys. 1 (5): 318. https://doi.org/10.1063/1.1745010.
Rieu, M., and G. Sposito. 1991. “Fractal fragmentation, soil porosity, and soil water properties: I. Theory.” Soil Sci. Soc. Am. J. 55 (5): 1231–1238. https://doi.org/10.2136/sssaj1991.03615995005500050006x.
Saint-Laurent, D., M. Hähni, J. St-Laurent, and F. Baril. 2010. “Comparative assessment of soil contamination by lead and heavy metals in riparian and agricultural areas (southern Québec, Canada).” Int. J. Environ. Res. Public Health 7 (8): 3100–3114. https://doi.org/10.3390/ijerph7083100.
Song, S., F. Li, J. Li, and Q. Liu. 2013. “Distribution and contamination risk assessment of dissolved trace metals in surface waters in the Yellow River Delta.” Hum. Ecol. Risk Assess. Int. J. 19 (6): 1514–1529. https://doi.org/10.1080/10807039.2012.708254.
Sun, H., M. M. Meerschaert, Y. Zhang, J. Zhu, and W. Chen. 2013. “A fractal Richards’ equation to capture the non-Boltzmann scaling of water transport in unsaturated media.” Adv. Water Resour. 52 (Nov): 292–295. https://doi.org/10.1016/j.advwatres.2012.11.005.
Tyler, S. W., and S. W. Wheatcraft. 1990. “Fractal processes in soil water retention.” Water Resour. Res. 26 (5): 1047. https://doi.org/10.1029/WR026i005p01047.
Wang, K., and R. Zhang. 2011. “Heterogeneous soil water flow and macropores described with combined tracers of dye and iodine.” J. Hydrol. 397 (1–2): 105–117. https://doi.org/10.1016/j.jhydrol.2010.11.037.
Wang, Q., R. Horton, and M. Shao. 2002. “Horizontal infiltration method for determining brooks-Corey model parameters.” Soil Sci. Soc. Am. J. 66 (6): 1733–1739. https://doi.org/10.2136/sssaj2002.1733.
Xu, T., I. D. Moore, and J. C. Gallant. 1993. “Fractals, fractal dimensions and landscapes—A review.” Geomorphology 8 (4): 245–262. https://doi.org/10.1016/0169-555X(93)90022-T.
Yakov, P., and D. Timlin. 1998. “Water transport in soils as in fractal media.” J. Hydrol. 204 (1–4): 98–107. https://doi.org/10.1016/S0022-1694(97)00110-8.
Ylva, P., H. M. Kristian, O. Lars, T. Mats, and E. Anja. 2008. “Use of a column leaching test to study the mobility of chlorinated HOCs from a contaminated soil and the distribution of compounds between soluble and colloid phases.” Chemosphere 71 (6): 1035–1042. https://doi.org/10.1016/j.chemosphere.2007.12.008.

Information & Authors

Information

Published In

Go to Journal of Hydrologic Engineering
Journal of Hydrologic Engineering
Volume 28Issue 2February 2023

History

Received: Dec 22, 2021
Accepted: Oct 14, 2022
Published online: Dec 1, 2022
Published in print: Feb 1, 2023
Discussion open until: May 1, 2023

Permissions

Request permissions for this article.

Authors

Affiliations

Ph.D. Student, College of Mechanics and Materials, Hohai Univ., No. 8 Fochengxi Rd., Nanjing, Jiangsu 211100, PR China. Email: [email protected]
Deshun Yin, Ph.D. [email protected]
Professor, College of Mechanics and Materials, Hohai Univ., No. 8 Fochengxi Rd., Nanjing, Jiangsu 211100, PR China (corresponding author). Email: [email protected]
Ph.D. Student, College of Mechanics and Materials, Hohai Univ., No. 8 Fochengxi Rd., Nanjing, Jiangsu 211100, PR China. Email: [email protected]
Guangjian Xiang [email protected]
Ph.D. Student, College of Mechanics and Materials, Hohai Univ., No. 8 Fochengxi Rd., Nanjing, Jiangsu 211100, PR China. Email: [email protected]

Metrics & Citations

Metrics

Citations

Download citation

If you have the appropriate software installed, you can download article citation data to the citation manager of your choice. Simply select your manager software from the list below and click Download.

View Options

Get Access

Access content

Please select your options to get access

Log in/Register Log in via your institution (Shibboleth)
ASCE Members: Please log in to see member pricing

Purchase

Save for later Information on ASCE Library Cards
ASCE Library Cards let you download journal articles, proceedings papers, and available book chapters across the entire ASCE Library platform. ASCE Library Cards remain active for 24 months or until all downloads are used. Note: This content will be debited as one download at time of checkout.

Terms of Use: ASCE Library Cards are for individual, personal use only. Reselling, republishing, or forwarding the materials to libraries or reading rooms is prohibited.
ASCE Library Card (5 downloads)
$105.00
Add to cart
ASCE Library Card (20 downloads)
$280.00
Add to cart
Buy Single Article
$35.00
Add to cart

Get Access

Access content

Please select your options to get access

Log in/Register Log in via your institution (Shibboleth)
ASCE Members: Please log in to see member pricing

Purchase

Save for later Information on ASCE Library Cards
ASCE Library Cards let you download journal articles, proceedings papers, and available book chapters across the entire ASCE Library platform. ASCE Library Cards remain active for 24 months or until all downloads are used. Note: This content will be debited as one download at time of checkout.

Terms of Use: ASCE Library Cards are for individual, personal use only. Reselling, republishing, or forwarding the materials to libraries or reading rooms is prohibited.
ASCE Library Card (5 downloads)
$105.00
Add to cart
ASCE Library Card (20 downloads)
$280.00
Add to cart
Buy Single Article
$35.00
Add to cart

Media

Figures

Other

Tables

Share

Share

Copy the content Link

Share with email

Email a colleague

Share