Collecting Particulate Matter and Particle-Bound Polycyclic Aromatic Hydrocarbons Using a Cylindrical Thermal Precipitator
Publication: Journal of Environmental Engineering
Volume 143, Issue 6
Abstract
Thermophoresis has been used to develop various thermal precipitators; however, their collection performance for ambient particulate matter (PM) with an aerodynamic diameter less than 10 μm () has been rarely reported, and the effect of the temperature gradient adopted in the precipitator on the evaporation loss of the organic fraction of collected particles has not been discussed to the authors’ knowledge. In this study, a cylindrical thermal precipitator consisting of two coaxially aligned cylinders with an annular space of 0.51 mm and a two-inlet impactor was designed for collecting . The effects of the sampling flow rate and temperature gradient on the collection efficiency were examined. The precipitator was also tested for its collection efficiency for particle-bound polycyclic aromatic hydrocarbons (PAHs). At a temperature gradient of and a flow rate of , the collection efficiency could reach 100% for PM with an electrical mobility diameter and decreased gradually to 70% as increased from 0.5 to 1.0 μm. For PM with , the collection efficiency increased due to impaction at the inlet. The collection efficiency increased with an increase in the temperature gradient or a decrease in the inlet flow rate. The semiempirical model could reasonably fit the collection efficiency curve of the precipitator. No significant evaporation loss of PAHs was found when the temperature of the cold cylinder surface was approximately 0°C. It was concluded that the thermal precipitator could be used to collect ambient fine PM with a size less than 0.5 μm, and the inlet impactor design could improve the collection efficiency for coarse particles.
Get full access to this article
View all available purchase options and get full access to this article.
Acknowledgments
Funding for this study was provided by the National Natural Science Foundation of China (41390240, 41571130010, and 41130754). The authors express their great appreciation to Dr. Arantzazu Eiguren-Fernandez and Dr. Raymond Coveney for their help in editing this article.
References
Alfaro-Moreno, E., et al. (2002). “Biologic effects induced in vitro by from three different zones of Mexico City.” Environ. Health Persp., 110(7), 715–720.
Araujo, J. A., and Nel, A. E. (2009). “Particulate matter and atherosclerosis: Role of particle size, composition and oxidative stress.” Part. Fibre Toxicol., 6(1), 24.
Azong-Wara, N., et al. (2009). “Optimisation of a thermophoretic personal sampler for nanoparticle exposure studies.” J. Nanopart. Res., 11(7), 1611–1624.
Azong-Wara, N., et al. (2013). “Design and experimental evaluation of a new nanoparticle thermophoretic personal sampler.” J. Nanopart. Res., 15(4), 1–12.
Becker, S., and Soukup, J. M. (2003). “Coarse (), fine (), and ultrafine air pollution particles induce/increase immune costimulatory receptors on human blood-derived monocytes but not on alveolar macrophages.” J. Toxicol. Environ. Health A, 66(9), 847–859.
Bein, K. J., and Wexler, A. S. (2014). “A high-efficiency, low-bias method for extracting particulate matter from filter and impactor substrates.” Atmos. Environ., 90, 87–95.
Bein, K. J., and Wexler, A. S. (2015). “Compositional variance in extracted particulate matter using different filter extraction techniques.” Atmos. Environ., 107, 24–34.
Bird, R. B., Stewart, W. E., and Lightfoot, E. N. (2002). Transport phenomena, 2nd Ed., Wiley, New York.
Bredl, J., and Grieve, T. W. (1951). “A thermal precipitator for the gravimetric estimation of solid particles in flue gases.” J. Sci. Instrum., 28(1), 21–23.
Broßell, D., et al. (2013). “A thermal precipitator for the deposition of airborne nanoparticles onto living cells—Rationale and development.” J. Aerosol Sci., 63, 75–86.
Dobbins, R. A., and Megaridis, C. M. (1987). “Morphology of flame-generated soot as determined by thermophoretic sampling.” Langmuir, 3(2), 254–259.
Gualtieri, M., et al. (2010). “Differences in cytotoxicity versus pro-inflammatory potency of different PM fractions in human epithelial lung cells.” Toxicol. in Vitro, 24(1), 29–39.
Hetland, R. B., et al. (2004). “Release of inflammatory cytokines, cell toxicity and apoptosis in epithelial lung cells after exposure to ambient air particles of different size fractions.” Toxicol. in Vitro, 18(2), 203–212.
Hinds, W. C. (1999). Aerosol technology: properties, behavior, and measurement of airborne particles, 2nd Ed., Wiley-Interscience, New York, 133–148.
Hu, M., et al. (2012). “Estimation of size-resolved ambient particle density based on the measurement of aerosol number, mass, and chemical size distributions in the winter in Beijing.” Environ. Sci. Technol., 46(18), 9941–9947.
Kethley, T. W., Gordon, M. T., and Orr, C., Jr. (1952). “A thermal precipitator for aerobacteriology.” Science, 116(3014), 368–369.
Kim, S., Jaques, P. A., Chang, M. C., Froines, J. R., and Sioutas, C. (2001). “Versatile aerosol concentration enrichment system (VACES) for simultaneous in vivo and in vitro evaluation of toxic effects of ultrafine, fine and coarse ambient particles—Part I: Development and laboratory characterization.” J. Aerosol Sci., 32(11), 1281–1297.
Leith, D., Miller-Lionberg, D., Casuccio, G., Lersch, T., Lentz, H., Marchese, A., and Volckens, J. (2014). “Development of a transfer function for a personal, thermophoretic nanoparticle sampler.” Aerosol Sci. Technol., 48(1), 81–89.
Marple, V. A., and Willeke, K. (1976). “Impactor design.” Atmos. Environ., 10(10), 891–896.
Messerer, A., Niessner, R., and Pöschl, U. (2003). “Thermophoretic deposition of soot aerosol particles under experimental conditions relevant for modem diesel engine exhaust gas systems.” J. Aerosol Sci., 34(8), 1009–1021.
Miller, A., Marinos, A., Wendel, C., King, G., and Bugarski, A. (2012). “Design optimization of a portable thermophoretic precipitator nanoparticle sampler.” Aerosol Sci. Technol., 46(8), 897–904.
Mohr, P. J., Taylor, B. N., and Newell, D. B. (2008). “CODATA recommended values of the fundamental physical constants: 2006.” J. Phys. Chem. Ref. Data, 37(3), 1187–1284.
Pope, C. A., III., and Dockery, D. W. (2006). “Health effects of fine particulate air pollution: lines that connect.” J. Air Waste Manage., 56(6), 709–742.
Sagot, B., Antonini, G., and Buron, F. (2009). “Annular flow configuration with high deposition efficiency for the experimental determination of thermophoretic diffusion coefficients.” J. Aerosol Sci., 40(12), 1030–1049.
Schlichting, H. (1979). Boundary-layer theory, 7th Ed., McGraw-Hill, New York.
Shen, G. F., et al. (2011). “Emissions of PAHs from indoor crop residue burning in a typical rural stove: Emission factors, size distributions, and gas-particle partitioning.” Environ. Sci. Technol., 45(4), 1206–1212.
Talbot, L., Cheng, R. K., Schefer, R. W., and Willis, D. R. (1980). “Thermophoresis of particles in a heated boundary-layer.” J. Fluid Mech., 101(04), 737–758.
Thayer, D., Koehler, K. A., Marchese, A., and Volckens, J. (2011). “A personal, thermophoretic sampler for airborne nanoparticles.” Aerosol Sci. Technol., 45(6), 744–750.
Tsai, C. J., and Lu, H. C. (1995). “Design and evaluation of a plate-to-plate thermophoretic precipitator.” Aerosol Sci. Technol., 22(2), 172–180.
Volckens, J., Dailey, L., Walters, G., and Devlin, R. B. (2009). “Direct particle-to-cell deposition of coarse ambient particulate matter increases the production of inflammatory mediators from cultured human airway epithelial cells.” Environ. Sci. Technol., 43(12), 4595–4599.
Wang, B., et al. (2013). “Properties and inflammatory effects of various size fractions of ambient particulate matter from Beijing on A549 and J774A.1 cells.” Environ. Sci. Technol., 47(18), 10583–10590.
Wang, B., Ou, Q. S., Tao, S., and Chen, D. R. (2012a). “Performance study of a disk-to-disk thermal precipitator.” J. Aerosol Sci., 52, 45–56.
Wang, B., Tao, S., and Chen, D. R. (2012b). “A cylindrical thermal precipitator with a particle size-selective inlet.” Aerosol Sci. Technol., 46(11), 1227–1238.
Zhang, J. J., and Smith, K. R. (2007). “Household air pollution from coal and biomass fuels in China: measurements, health impacts, and interventions.” Environ. Health Persp., 115(6), 848–855.
Information & Authors
Information
Published In
Copyright
©2017 American Society of Civil Engineers.
History
Received: Jul 31, 2016
Accepted: Dec 2, 2016
Published ahead of print: Feb 21, 2017
Published online: Feb 22, 2017
Published in print: Jun 1, 2017
Discussion open until: Jul 22, 2017
Authors
Metrics & Citations
Metrics
Citations
Download citation
If you have the appropriate software installed, you can download article citation data to the citation manager of your choice. Simply select your manager software from the list below and click Download.