TECHNICAL PAPERS
Nov 17, 2010

Ceramic Filters Impregnated with Silver Nanoparticles for Point-of-Use Water Treatment in Rural Guatemala

Publication: Journal of Environmental Engineering
Volume 137, Issue 6

Abstract

The technological performance and social acceptance of ceramic water filters impregnated with silver nanoparticles for point-of-use water treatment were investigated in the laboratory and in the field in the Guatemalan highland community of San Mateo Ixtatán. In the laboratory, filters were constructed with clay and sawdust collected from the Guatemalan community and were tested to determine the effects of percent sawdust and silver nanoparticle treatment on the transport and removal of E. coli. For ceramic filters without silver treatment, size-exclusion and/or sorption is the mechanism of removal and a lower mass-percent sawdust corresponds to greater bacteria removal. The addition of silver nanoparticles to the ceramic filters improved the performance for all mass percentages of sawdust relative to filter media without nanoparticle treatment. Filters with higher porosity achieved higher bacteria removal than those with lower porosity, suggesting an increase in burnable material percentage is advantageous, assuming structural integrity is not compromised. Subsequent to laboratory testing, ceramic filters were manufactured with local materials and labor in San Mateo Ixtatán, Guatemala, and distributed to 62 households in this peri-urban community. The study participants were randomly divided into two groups, and filters were tested periodically over 23 months or 12 months. Filtered effluent samples were tested for turbidity reduction, bacteria removal, and silver leaching. Over the course of the study, the average percent reduction in total coliforms and E. coli was 87% and 92%, respectively. The average effluent turbidity was 0.18 nephelometric turbidity units (NTUs) and average effluent concentration of ionic silver was 0.02mg/L (below the U.S. EPA standard of 0.1mg/L). Filters distributed to the second study group consistently performed better than the first study group as manufacturing techniques improved and contact with researchers increased. Overall, users were satisfied with the filters, citing them as easy to use and maintain while improving water quality. The findings of this study suggest that locally manufactured ceramic filters can significantly improve the microbiological quality of water when used as a point-of-use water-treatment technology.

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Acknowledgments

This research was supported by the Environmental Sustainability Program of the U.S. National Science Foundation (NSFCBET 651996). The authors thank the Ixtatán Foundation for community-level support of this research, E. Fauss and N. Swami for providing the TEM image of silver nanoparticles (Fig. 1), and H. Yu, K. Kline, R. Massey, and D. Restivo for assistance during the collection and analysis of our field data.

References

Bartelt-Hunt, S. L., Burns, S. E., and Smith, J. A. (2003). “Nonionic organic solute sorption to two organobentonites as a function of organic-carbon content.” J. Colloid Interface Sci., 266(2), 251–258.
Bielefeldt, A. R., et al. (2010). “Removal of virus to protozoan sized particles in point-of-use ceramic water filters.” Water Res., 44(5), 1482–1488.
Bielefeldt, A. R., Kowalski, K., and Summers, R. S. (2009). “Bacterial treatment effectiveness of point-of-use ceramic water filters.” Water Res., 43(14), 3559–3565.
Brown, J., Sobsey, M. D., and Loomis, D. (2008). “Local drinking water filters reduce diarrheal disease in Cambodia: A randomized, controlled trial of the ceramic water purifier.” Trop. Med. Int. Health, 79(3), 394–400.
Central Intelligence Agency (CIA). (2003). “The world factbook—Guatemala.” 〈http://www.cia.gov/cia/publications/factbook/geos/gt.html〉 (Feb. 22, 2008).
Clasen, T., et al. (2007). “Interventions to improve water quality for preventing diarrhoea: Systematic review and meta-analysis.” Br. Med. J., 334(7597), 782.
Clasen, T., Nadakatti, S., and Menon, S. (2006). “Microbiological performance of a water treatment unit designed for household use in developing countries.” Trop. Med. Int. Health, 11(9), 1399–1405.
Hach. (2003). Silver colorimetric method: Method 8120 DR/4000 procedure, 11th Ed., Hach Company, Loveland, CO.
Lantagne, D. S. (2001). “Investigation of the Potters for Peace colloidal silver impregnated ceramic filter.” United States Aid for International Development (USAID), 79.
Nath, K., Bloomfield, S., and Jones, M. (2006). “Household water storage, handling and point-of-use treatment.” Review commissioned by International Scientific Forum on Home Hygene (IFH), 〈http://www.ifh-homehygiene.org〉.
Oyanedel-Craver, V., and Smith, J. A. (2008). “Sustainable colloidal-silver-impregnated ceramic filter for point-of-use water treatment.” Environ. Sci. Technol., 42(3), 927–933.
Rayner, J. (2009). “Current practices in manufacturing of ceramic pot filters for water treatment water.” M.S. thesis, Engineering and Development Centre (WEDC), Loughborough Univ., Loughborough, UK.
Sherwood, J. L., et al. (2003). “Analysis of bacterial random motility in a porous medium using magnetic resonance imaging and immunomagnetic labeling.” Environ. Sci. Technol., 37(4), 781–785.
Sondi, I., Goia, D. V., and Matijevic, E. (2003). “Preparation of highly concentrated stable dispersions of uniform silver nanoparticles.” J. Colloid Interface Sci., 260(1), 75–81.
Sondi, I., and Salopek-Sondi, B. (2004). “Silver nanoparticles as antimicrobial agent: A study on E. coli as a model for gram-negative bacteria.” J. Colloid Interface Sci., 275(1), 177–182.
United Nations (UN). (2005). “UN millennium development goals.” 〈http://www.un.org/milleniumgoals/〉 (Nov. 25, 2008).
United Nations Environmental Programme. (2009). “Human impact 2002.” Globalis. 〈http://globalis.gvu.unu.edu/〉 (Apr. 3, 2009).
van Halem, D., et al. (2009). “Assessing the sustainability of the silver-impregnated ceramic pot filter for low-cost household drinking water treatment.” Phys. Chem. Earth, 34(1–2), 36–42.
Vigeant, M. A., Ford, R. M., Wagner, M., and Tamm, L. K. (2002). “Reversible and irreversible adhesion of motile Escherichia coli cells analyzed by total internal reflection aqueous fluorescence microscopy.” Appl. Environ. Microbiol., 68(6), 2794–2801.
World Health Organization (WHO). (2003). WHO guidelines for drinking water quality, 3rd Ed., World Health Organization, Geneva.
World Health Organization (WHO). (2008). “Drinking water.” 〈http://whqlibdoc.who.int/publications/2008/9789241563673_part3_eng.pdf〉 (Apr. 17, 2009).

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Information

Published In

Go to Journal of Environmental Engineering
Journal of Environmental Engineering
Volume 137Issue 6June 2011
Pages: 407 - 415

History

Received: Mar 24, 2010
Accepted: Nov 5, 2010
Published online: Nov 17, 2010
Published in print: Jun 1, 2011

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Authors

Affiliations

Erin N. Kallman
Graduate Research Assistant, Dept. of Civil and Environmental Engineering, Univ. of Virginia, P.O. Box 400742, Charlottesville, VA 22904-4742.
Vinka A. Oyanedel-Craver, A.M.ASCE
Assistant Professor, Dept. of Civil and Environmental Engineering, Univ. of Rhode Island, Kingston, RI 02881.
James A. Smith, M.ASCE [email protected]
Dept. of Civil and Environmental Engineering, Univ. of Virginia, P.O. Box 400742, Charlottesville, VA 22904-4742 (corresponding author). E-mail: [email protected]

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