How Competitive Hydration between C3A and C3S in the Fast Dissolution Stage Affects the Hydration of Low-Heat Portland Cement Blended Pastes
Publication: Journal of Materials in Civil Engineering
Volume 36, Issue 5
Abstract
Xinjiang has a temperature difference of 20°C between day and night, interannual temperature difference of 50°C, the control of the temperature cracks in mass concrete becomes difficult. Although low-heat portland () cement concrete containing fly ash (FA) can reduce hydration heat, the mismatch between its mechanical and thermal properties is still not fully resolved. An attempt to explore the effect of FA on the competitive hydration reaction of and at super-early ages, and how this effect changes the physical and chemical properties of hardened cement pastes by electrical resistivity and zeta potential and common microstructure test methods, and to provide a theoretical basis for optimization of mechanical and thermal properties of cement concrete with FA. Results showed that in the fast dissolution stage, a numerous ions and a very small amount of ions were formed, and incorporating 20%, 30%, 40% FA primarily inhibited the hydration and the generation, resulting in the generation time of AFt in comparison with pure cement, respectively, delayed by 44%, 140%, and 524%. This phenomenon decreased the nucleation and crystallization growth rate of AFt and in the induction stage, and reduced the consumption of gypsum in the acceleration stage. Hence, monosulfoaluminate did not exist for pastes with more than 30% FA, and the number of particles involved in the reaction for the cement stone with 20%, 30%, and 40% FA decreased by 4.0%, 46.5%, and 52.0% in the deceleration stage compared with the pure cement. The research results can provide a theoretical reference for modifying chemical properties of FA to meet the matching of mechanical strength and thermal of cement.
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Data Availability Statement
All data that support the findings of this study are available from the corresponding author upon reasonable request.
Acknowledgments
The authors sincerely appreciate the support from the Outstanding Youth Science Foundation of Natural Science Foundation of Xinjiang Uygur Autonomous Region, China (Grant No. 2022D01E44), the Teacher Training Program of the College of Hydraulic and Civil Engineering in Xinjiang Agricultural University, China (Grant No. ZDSYS–JS–2021–12), and the 2022 Postgraduate Hydraulic Engineering Key Discipline Research Project (Grant No. ZDSYS–YJS–2022–12).
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Journal of Materials in Civil Engineering
Volume 36 • Issue 5 • May 2024
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© 2024 American Society of Civil Engineers.
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Received: Jun 9, 2023
Accepted: Oct 27, 2023
Published online: Feb 24, 2024
Published in print: May 1, 2024
Discussion open until: Jul 24, 2024
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