Resuspension of Mercury-Contaminated Sediments from an In-Lake Industrial Waste Deposit
Publication: Journal of Environmental Engineering
Volume 135, Issue 7
Abstract
The resuspension and transport of particulate mercury from a nearshore industrial waste deposit to the pelagic zone of Onondaga Lake, N.Y., was investigated using an array of sediment traps radiating from the deposit, and quantified through application of a steady-state mass balance model. Time-averaged downward fluxes of suspended solids and decreased in the offshore direction, indicating a nearshore source. Strong temporal variations in resuspension were documented and were linked to the dynamics of wind-driven wave action, as quantified by a validated surface wave model. A simple steady-state model of offshore transport from the resuspension zone, which assumes a balance between offshore transport and settling, was used to analyze sediment trap data. The resulting larger, and likely more accurate, estimate of resuspension represents the dominant contemporary source to the water column. This result supports the planned remediation of this source as a part of a Superfund cleanup project.
Get full access to this article
View all available purchase options and get full access to this article.
Acknowledgments
Support for this study was provided by the U.S. Environmental Protection Agency (Grant No. UNSPECIFIEDCR-083091201-0). This is contribution No. UNSPECIFIED259 of the Upstate Freshwater Institute.
References
Benoit, J. M., Gilmour, C. C., and Mason, R. P. (2001). “The influence of sulfide on solid-phase mercury bioavailability for methylation by pure cultures of Desulfobulbus propionicus (1pr3).” Environ. Sci. Technol., 35(1), 127–132.
Bloesch, J. (1982). “Inshore-offshore sedimentation differences resulting from resuspension in the eastern basin of Lake Erie.” Can. J. Fish. Aquat. Sci., 39(5), 748–759.
Bloesch, J. (1995). “Mechanisms, measurement and importance of sediment resuspension in lakes.” Mar. Freshwater Res., 46(1), 295–304.
Bloesch, J. (1996). “Towards a new generation of sediment traps and a better measurement/understanding of settling particulate flux in lakes and oceans: A hydrodynamic protocol.” Aquat. Sci., 58(4), 283–296.
Bloesch, J., and Uehlinger, U. (1986). “Horizontal sedimentation differences in a eutrophic Swiss Lake.” Limnol. Oceanogr., 31(5), 1094–1109.
Bloom, N. W., and Effler, S. W. (1990). “Seasonal variability in the mercury speciation of Onondaga Lake, NY.” Water, Air, Soil Pollut., 53(3–4), 251–265.
Bogdan, J. J., Budd, J. W., Eadie, B. J., and Hornbuckle, K. C. (2002). “The effect of a large resuspension event in southern Lake Michigan on the short-term cycling of organic contaminants.” J. Great Lakes Res., 28(3), 338–351.
Brookes, J. D., Antenucci, J., Hipsey, M., Burch, M. D., Ashbolt, N. J., and Ferguson, C. (2004). “Fate and transport of pathogens in lakes and reservoirs.” Environ. Int., 30(5), 741–759.
Dean, R. G., and Dalrymple, R. A. (1984). Water wave mechanics for engineers and scientists, Prentice-Hall, Englewood Cliffs, N.J.
Driscoll, C. T., et al. (2007). “Mercury contamination in forest and freshwater ecosystems in the northeastern United States.” BioScience, 57(1), 17–28.
Effler, S. W. (1996). Limnological and engineering analysis of a polluted urban lake: Prelude to environmental management of Onondaga Lake, New York, Springer, New York.
Effler, S. W., Gelda, R. K., Field, S. D., Effler, A. J. P., Wallenberg, E. B., and Matthews, D. A. (2005). “Changes in primary production in Onondaga Lake, NY: Magnitude, metrics, and drivers.” Lake Reserv. Manage., 21(1), 61–72.
Effler, S. W., and Matthews, D. A. (2003). “Impacts of a soda ash facility on Onondaga Lake and the Seneca River, NY.” Lake Reserv. Manage., 19(4), 285–306.
Effler, S. W., and Matthews, D. A. (2004). “Sediment resuspension and drawdown in a water supply reservoir.” J. Am. Water Resour. Assoc., 40(1), 251–264.
Effler, S. W., Matthews-Brooks, C. M., and Driscoll, C. T. (2001). “Changes in deposition of phytoplankton constituents in a polluted lake.” Environ. Sci. Technol., 35(15), 3082–3088.
Effler, S. W., Perkins, M. G., and Johnson, D. L. (1998). “The optical water quality of Cannonsville Reservoir: Spatial and temporal patterns, and the relative roles of phytoplankton and inorganic tripton.” Lake Reserv. Manage., 14(2–3), 238–253.
Gailani, J., Ziegler, C. K., and Lick, W. (1991). “The transport of sediments in the Lower Fox River.” J. Great Lakes Res., 17(4), 479–494.
Gloor, M., Wuest, A., and Munnich, M. (1994). “Benthic boundary mixing and resuspension induced by internal seiches.” Hydrobiologia, 284(1), 59–68.
James, R. T., Martin, J., Wool, T., and Wang, P. F. (1997). “A sediment resuspension and water quality model of Lake Okeechobee.” J. Am. Water Resour. Assoc., 33(3), 661–680.
James, W. F., and Barko, J. W. (1993). “Sediment resuspension, redeposition, and focusing in a small dimictic reservoir.” Can. J. Fish. Aquat. Sci., 50(5), 1023–1028.
Jin, K.-R., and Ji, Z.-G. (2004). “Case study: Modeling of sediment transport and wind-wave impact in Lake Okeechobee.” J. Hydraul. Eng., 130(11), 1055–1067.
LeFevre, N. M., and Lewis, G. D. (2003). “The role of resuspension in enterococci distribution in water at an urban beach.” Water Sci. Technol., 47(3), 205–210.
Linge, K. L., and Oldham, C. E. (2002). “Arsenic remobilization in a shallow lake: the role of sediment resuspension.” J. Environ. Qual., 31(3), 822–828.
Luettich, R. A., Harleman, D. R. F., and Somlyody, L. (1990). “Dynamic behavior of suspended sediment concentrations in a shallow lake perturbed by episodic wind events.” Limnol. Oceanogr., 35(5), 1050–1067.
Martin, J. L., and McCutcheon, S. C. (1999). Hydrodynamics and transport for water quality modeling, Lewis, Boca Raton, Fla.
Matthews, D. A., and Effler, S. W. (2006). “Long-term assessment of the oxygen resources of a recovering urban lake, Onondaga Lake, NY.” Lake Reserv. Manage., 22(1), 19–32.
Matthews, D. A., Effler, S. W., O’Donnell, S. M., Driscoll, C. T., and Matthews, C. M. (2008). “Electron budgets for the hypolimnion of a recovering urban lake, 1989–2004: Response to changes in organic carbon deposition and availability of electron acceptors.” Limnol. Oceanogr., 53(2), 743–759.
Mehta, A. J., Hayter, E. J., Parker, W. R., Krone, R. B., and Teeter, A. M. (1989). “Cohesive sediment transport. 1: Process description.” J. Hydraul. Eng., 115(8), 1076–1093.
New York State Department of Environmental Conservation (NYSDEC). (2004). “Onondaga Lake bottom subsite of the Onondaga Lake superfund site, Syracuse, New York.” Technical Rep., New York State Department of Environmental Conservation, Albany, N.Y.
Rosa, F., Bloesch, J., and Rathke, D. E. (1991). “Sampling the settling and suspended particulate matter (SPM).” Handbook of techniques of aquatic sediment sampling, A. Mudroch and S. C. Macknight, eds., CRC, Ann Arbor, Mich., 97–130.
Schwab, D. J., Bennett, J. R., Liu, P. C., and Donelan, M. A. (1984). “Application of a simple numerical wave prediction model to Lake Erie.” J. Geophys. Res., 89(C3), 3586–3592.
Sharpe, C. W. (2004). “Mercury dynamics of Onondaga Lake and adjacent wetlands.” MS thesis, Syracuse Univ., Syracuse, N.Y.
TAMS Consultants, Inc. (2002). “Onondaga Lake remedial investigation.” Document Prepared by Exponent, Bellevue, WA for Honeywell, Revised Ed., New York State Department of Environmental Conservation, Albany, N.Y.
United States Environmental Protection Agency (USEPA). (1973). “Report of mercury source investigation: Onondaga Lake, New York and Allied Chemical Corporation, Solvay, New York.” Rep., National Field Investigation Center, Cincinnati.
Weyhenmeyer, G. A., Meili, M., and Pierson, D. C. (1995). “A simple method to quantify sources of settling particles in lakes: Resuspension versus new sedimentation of material from planktonic production.” Mar. Freshwater Res., 46(1), 223–231.
Wodka, M. C., Effler, S. W., and Driscoll, C. T. (1985). “Phosphorus deposition from the epilimnion of Onondaga Lake.” Limnol. Oceanogr., 30(4), 833–843.
Womble, R. N., Driscoll, C. T., and Effler, S. W. (1996). “Calcium carbonate deposition in polluted Onondaga Lake, New York, U.S.A.” Water Res., 30(9), 2139–2147.
Yin, C., and Johnson, D. L. (1984). “An individual particle analysis and budget study of Onondaga Lake sediments.” Limnol. Oceanogr., 29(6), 1193–1201.
Information & Authors
Information
Published In
Copyright
© 2009 ASCE.
History
Received: Jun 28, 2007
Accepted: Dec 9, 2008
Published online: Jun 15, 2009
Published in print: Jul 2009
Authors
Metrics & Citations
Metrics
Citations
Download citation
If you have the appropriate software installed, you can download article citation data to the citation manager of your choice. Simply select your manager software from the list below and click Download.