TECHNICAL PAPERS
Feb 1, 1999

Dioxins and Furans Urban Runoff

Publication: Journal of Environmental Engineering
Volume 125, Issue 2

Abstract

Urban runoff samples were collected in a 1-year period in the Santa Monica Bay watershed during both dry and storm periods and analyzed for polychlorinated dioxins, polychlorinated furans, and polychlorinated naphthalenes. Trace concentrations were found in nearly all of the samples collected. During storms polychlorinated dioxin and polychlorinated furan concentrations peaked. The congener and isomer profiles resemble profiles found in lake sediments and rainwater more than they resemble profiles found in urban sources such as dioxins from incinerators or dioxins in contaminated commercial products. Runoff from open land use had lower concentrations than runoff from developed land uses.

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References

1.
Amendola, G., et al. ( 1989). “The occurrence and fate of PCDDs and PCDFs in five bleached kraft pulp and paper mills.” Chemosphere, 18(1-6), 1181–1188.
2.
Asplund, K., Mar, B. W., and Ferguson, J. F. (1982). “Total suspended solids in highway runoff in Washington State.”J. Envir. Engrg. Div., ASCE, 108, 391–404.
3.
Atkinson, R. ( 1991). “Atmospheric lifetimes of dibenzo-p-dioxins and dibenzofurans.” Sci. Total Envir., Amsterdam, 104(1), 17–33.
4.
Bay, S. M., Greenstein, D. J., Lau, D. J., Stenstrom, S.-L., and Kelley, M. K. ( 1996). “Toxicity of dry weather flow from the Santa Monica Bay watershed.” Bull. of Southern California Acad. Sci., 95, 33–45.
5.
Broman, D., Naf, C., Zebuhr, Y., and Lexen, K. ( 1989). “The composition, distribution and flux of PCDDs and PCDFs in settling particulate matter (SPM)–a sediment trap study in the northern Baltic.” Chemosphere, 19(1-6), 445–450.
6.
Bumpus, J. A., Tien, M., Wright, D., and Aust, S. D. ( 1985). “Oxidation of persistent environmental pollutants by a white rot fungus.” Science, 228, 1434–1436.
7.
Buser, H. R., Bosshardt, H.-P, Rappe, C., and Lindahl, R. ( 1978). “Identification of polychlorinated dibenzofuran isomers in fly ash and PCB pyrolyses.” Chemosphere, 7(5), 419–429.
8.
Crummett, W. B., and Stehl, R. H. ( 1973). “Determination of chlorinated dibenzo-p-dioxins and dibenzofurans in various materials.” Envir. Health Perspective, 5, 15–25.
9.
Czuczwa, J. M., and Hites, R. A. ( 1984). “Environmental fate of combustion-generated polychlorinated dioxins and furans.” Envir. Sci. and Technol., 18(6), 444–450.
10.
Czuczwa, J. M., and Hites, R. A. ( 1985). “Historical record of polychlorinated dioxins and furans in Lake Huron sediments.” Chlorinated dioxins and dibenzofurans in the total environment II, L. H. Keith, C. Rappe, and G. Choudhary, eds., Butterworth's, Boston, 59–63.
11.
Czuczwa, J. M., and Hites, R. A. ( 1986a). “Sources and fate of PCDD and PCDF.” Chemosphere, 15(9-12), 1417–1420.
12.
Czuczwa, J. M., and Hites, R. A. ( 1986b). “Airborne dioxins and dibenzofurans: Sources and fates.” Envir. Sci. and Technol., 20(2), 195–200.
13.
Czuczwa, J. M., NcVeety, B. D., and Hites, R. A. ( 1984). “Polychlorinated dibenzo-p-dioxins and dibenzofurans in sediments from Siskiwit Lake, Isle Royale.” Science, 226, 568–569.
14.
Czuczwa, J. M., Niessen, F., and Hites, R. A. ( 1985). “Historical record of polychlorinated dibenzo-p-dioxins and dibenzofurans in Swiss lake sediments.” Chemosphere, 14(9), 1175–1179.
15.
Eganhouse, R. P., Simoneit, B. R. T., and Kaplan, I. R. ( 1981). “Extractable organic matter in urban stormwater runoff. 2. Molecular characterization.” Envir. Sci. and Technol., 15, 315–326.
16.
Fam, S., Stenstrom, M. K., and Silverman, G. (1987). “Hydrocarbons in urban runoff.”J. Envir. Engrg., ASCE, 113(5), 1032–1046.
17.
Fiedler, H., Hutzinger, O., and Timms, C. W. ( 1990). “Dioxins: Sources of environmental load and human exposure.” Toxicological and Envir. Chem., 29(3), 157–234.
18.
Fisher, T. S. ( 1998). “Dioxins, furans, and polychlorinated furans in urban runoff,” MS thesis, Department of Civil and Environmental Engineering, University of California, Los Angeles.
19.
Hites, R. A. ( 1990). “Environmental behavior of chlorinated dioxins and furans.” Acc. Chem. Res., 23(6), 194–201.
20.
Hoffman, E. J., Mills, G. L., Latimer, J. S., and Quinn, J. G. ( 1984). “Urban runoff as a source of polycyclic aromatic hydrocarbons to coastal waters.” Envir. Sci. and Technol., 18, 580–587.
21.
Hunt, G. T., and Maisel, B. E. ( 1992). “Atmospheric concentrations of PCDDs/PCDFs in Southern California.” J. Air Waste Mgmt. Assoc., 42(5), 672–680.
22.
Ligon Jr., W. V., Dorn, S. B., and May, R. J. ( 1989). “Chlorodibenzofuran and chlorodibenzo-p-dioxin levels in Chilean mummies dated to about 2,800 years before the present.” Envir. Sci. and Technol., 23(10), 1286–1290.
23.
Marklund, S., et al. ( 1986). “Determination of PCDDs and PCDFs in incineration samples and pyrolytic products.” Chlorinated dioxins and dibenzofurans in perspective, C. Rappe, G. Choudhary, and L. H. Keith, eds., Lewis, Chelsea, Mich., 79–82.
24.
Marklund, S., et al. ( 1990). “Emissions of PCDDs and PCDFs in gasoline and diesel fueled cars.” Chemosphere, 20(5), 553–561.
25.
North Atlantic Treaty Organization, Committee on the Challenges of Modern Society (NATO/CCMS). ( 1988a). “Pilot study on international information exchange on dioxins and related compounds.” International Toxicity Equivalency Factor (I-TEF) Method of Risk Assessment for Complex Mixtures of Dioxins and Related Compounds, Rep. No 176, NATO, Brussels.
26.
North Atlantic Treaty Organization, Committee on the Challenges of Modern Society (NATO/CCMS). ( 1988b). “Pilot study on international information exchange on dioxins and related compounds.” Scientific basis for the Development of International Toxicity Equivalency Factor (I-TEF) Method of Risk Assessment for Complex Mixtures of Dioxins and Related Compounds, Rep. No. 178, NATO, Brussels.
27.
Oberg, L. G., and Rappe, C. ( 1992). “Biochemical formation of PCDD/Fs from chlorophenols.” Chemosphere, 25(1-2), 49–52.
28.
Olie, K., Vermeulen, P. L., and Hutzinger, O. ( 1977). “Chlorodibenzo-p-dioxins and chlorodibenzofurans are trace components of fly ash and flue gas of some municipal incinerators in the Netherlands.” Chemosphere, 6(8), 455–459.
29.
Pitt, R., Field, R., Lalor, M., and Brown, M. ( 1995). “Urban stormwater toxic pollutants: assessment, sources and treatability.” Water Envir. Res., 67(3), 260–274.
30.
Podoll, R. T., Jaber, H. M., and Mill, T. ( 1986). “Tetrachlorodibenzodioxin: Rates of volatilization and photolysis in the environment.” Envir. Sci. and Technol., 20(5), 490–492.
31.
Rappe, C., Buser, H. R., Stalling, D. L., Smith, L. M., and Dougherty, R. C. ( 1981). “Identification of polychlorinated dibenzofurans in environmental samples.” Nature, 292, 524–526.
32.
Rappe, C., Gara, A., and Buser, H. R. ( 1978). “Identification of polychlorinated dibenzofurans (PCDFs) in commercial chlorophenol formulations.” Chemosphere, 7(12), 981–991.
33.
Rappe, C., Marklund, S., Kjeller, L.-O., and Lindskog, A. ( 1989). “Long-range transport of PCDDs and PCDFs on airborne particles.” Chemosphere, 18(1-6), 1283–1290.
34.
Sartor, J. D., Boyd, G. B., and Agardy, F. J. ( 1974). “Water pollution aspects of street surface contaminants.” J. Water Pollution Control Fed., 46, 458–467.
35.
Schecter, A., Dekin A., Weerasinghe, N. C. A., Arghestani, S., and Gross, M. L. ( 1988). “Sources of dioxins in the environment: A study of PCDDs and PCDFs in ancient, frozen Eskimo tissue.” Chemosphere, 17(4), 627–631.
36.
Stenstrom, M. K., Silverman, G. S., and Bursztynsky, T. A. (1984). “Oil and grease in urban stormwaters.”J. Envir. Engrg., ASCE, 110(1), 58–72.
37.
Stieglitz, L., Zwick, G., Beck, J., Roth, W., and Vogg, H. ( 1989). “On the de-nova synthesis of PCDD/PCDF on fly ash of municipal waste incinerators.” Chemosphere, 18(1-6), 1219–1226.
38.
Swansen, S. E. ( 1988). “Dioxins in the beach plant: a study of the occurrence and formation of polychlorinated dibenzofurans and polychlorinated dibenzo-p-dioxins in the chlorine bleaching of wood pulp,” PhD dissertation, Institute of Environmental Chemistry, University of Umea, Umea, Sweden.
39.
Whipple, J. A., and Hunter, J. V. ( 1979). “Petroleum hydrocarbons in urban runoff.” Water Resour. Bull., 15, 1096–1105.
40.
Wong, K., Strecker, E. W., and Stenstrom, M. K. (1997). “A Geographic Information System to estimate stormwater pollutant mass loadings.”J. Envir. Engrg., ASCE, 123(8), 737–745.

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Published In

Go to Journal of Environmental Engineering
Journal of Environmental Engineering
Volume 125Issue 2February 1999
Pages: 185 - 191

History

Received: Oct 1, 1997
Published online: Feb 1, 1999
Published in print: Feb 1999

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Authors

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Fellow, ASCE
Civ. and Envir. Engrg. Dept., Univ. of California, Los Angeles, 4173 Engineering I, Los Angeles, CA 90095-1593.
USFDA, 200 C St. S.W., Washington, DC 20204; formerly, Haz. Mat. Lab., California Dept. of Toxic Substances Control, Room 515, 2151 Berkeley Way, Berkeley, CA 94704.
Deputy Dir., Sci., Pollution Prevention and Technol. Program, California Dept. of Toxic Substances Control, Room 515, 2151 Berkeley Way, Berkeley, CA.
Civ. and Envir. Engrg. Dept., Univ. of California, Los Angeles, 4173 Engineering I, Los Angeles, CA.

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